The only solution that worked for my particular setup was to delete the following two files (After making sure all Chrome Windows/tabs & processes are closed)
“Web Data” and “Web Data-journal” files from the following location on my Windows7 machine:
C:\Users\[Enter your username here]\AppData\Local\Google\Chrome\User Data\Default
Although this solution was posted back in 2011, it still worked for my problem and resolved it without further tinkering.
Solution Source: http://akdora.wordpress.com/2011/11/03/solution-your-profile-could-not-be-opened-correctly-in-chrome/
P.S. I saw other solutions that suggested deleting your whole Chrome data folders & their contents. Make sure you backup your Chrome bookmarks and a list of your current extensions if you decide to go that route so you won't have to lose any of your stuff.
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